Title Information
Title
Experimental Constraints on the geochemical processing planetary interiors: Noble gases and spinel spectroscopy
Name: Personal
Name Part
Jackson, Colin
Role
Role Term: Text
creator
Origin Information
Copyright Date
2015
Physical Description
Extent
13, 301 p.
digitalOrigin
born digital
Note
Thesis (Ph.D. -- Brown University (2015)
Name: Personal
Name Part
Parman, Stephen
Role
Role Term: Text
Director
Name: Personal
Name Part
Cooper, Reid
Role
Role Term: Text
Reader
Name: Personal
Name Part
Saal, Alberto
Role
Role Term: Text
Reader
Name: Personal
Name Part
Mukhopadhyay, Sujoy
Role
Role Term: Text
Reader
Name: Personal
Name Part
Parmentier, Marc
Role
Role Term: Text
Reader
Name: Corporate
Name Part
Brown University. Geological Sciences
Role
Role Term: Text
sponsor
Genre (aat)
theses
Abstract
The first three chapters of this thesis are focused on experimental determinations of noble gas solubility in a variety of materials relevant to partial melting of the mantle and subduction. Combined, these chapters represent an experimental exploration of the deep noble gas cycle. In the first chapter, we show that helium, neon, and argon are strongly incompatible in upper mantle minerals. Further, we demonstrate that helium solubility in olivine is insensitive to changes in common point defect concentrations, suggesting helium is primarily incorporated onto interstitial sites. Application of helium solubility data to mantle melting models indicates that melting residues will have decreased He/(U+Th), and, with time, radiogenic helium isotopic signatures. The second two chapters focus on the mineralogic controls on noble gas recycling. Specifically, we quantify noble gas solubility in a wide range of minerals with lattice ring structures. We show that minerals with ring structures have a strong, but variable, affinity for helium, and thus, may facilitate recycling of noble gases. We further show that ring structure minerals tend to favor smaller radii noble gases. The final chapter is focused on determining the factors that control visible to near-infrared reflectance spectra of iron-bearing aluminate spinels. This chapter is motivated by the recent remote sensing detections of spinel-rich deposits on the Moon and seeks to provide additional geologic context for these spinels. To this end, we synthesized a series of spinels with variable amounts of iron under lunar-like redox conditions. By controlling point defect chemistry, we demonstrate that absorption bands near ~1000 nm in spinel are particularly sensitive to the abundance octahedral, ferrous iron, which is primarily controlled by cooling rate in natural systems. Accounting for geologic cooling rates, we conclude that 1) the spinels associated with central peaks and basin walls are very magnesian (~6 wt. % FeOt) and 2) the pyroclastic spinels associated with Sinus Aestuum either are ferric iron-rich or cooled very rapidly, possibly in the absence of an extensive vapor cloud.
Subject
Topic
noble gases
Subject (FAST) (authorityURI="http://id.worldcat.org/fast", valueURI="http://id.worldcat.org/fast/938685")
Topic
Gases, Rare
Subject (FAST) (authorityURI="http://id.worldcat.org/fast", valueURI="http://id.worldcat.org/fast/940343")
Topic
Geochemistry
Subject (FAST) (authorityURI="http://id.worldcat.org/fast", valueURI="http://id.worldcat.org/fast/1129958")
Topic
Spinel
Record Information
Record Content Source (marcorg)
RPB
Record Creation Date (encoding="iso8601")
20150601
Language
Language Term: Code (ISO639-2B)
eng
Language Term: Text
English
Identifier: DOI
10.7301/Z0CJ8BVC
Access Condition: rights statement (href="http://rightsstatements.org/vocab/InC/1.0/")
In Copyright
Access Condition: restriction on access
Collection is open for research.
Type of Resource (primo)
dissertations