Title Information
Title
Chemical and Thermochemical Properties of Graphene Oxide Based Materials: Safety Implications and Applications
Name: Personal
Name Part
qiu, yang
Role
Role Term: Text
creator
Origin Information
Copyright Date
2015
Physical Description
Extent
xvi, 154 p.
digitalOrigin
born digital
Note
Thesis (Ph.D. -- Brown University (2015)
Name: Personal
Name Part
Hurt, Robert
Role
Role Term: Text
Director
Name: Personal
Name Part
Kane, Agnes
Role
Role Term: Text
Director
Name: Personal
Name Part
Kane, Agnes
Role
Role Term: Text
Reader
Name: Personal
Name Part
Kulaots, Indrek
Role
Role Term: Text
Reader
Name: Corporate
Name Part
Brown University. ENGINEERING: Fluids and Thermal Sciences
Role
Role Term: Text
sponsor
Genre (aat)
theses
Abstract
The successful application of new materials requires good understanding of their basic properties which govern their behaviors during manufacturing, processing, storage and disposal. Graphene based materials as an emerging family of carbon materials with promising mechanical, electrical and thermal properties have been believed to be “game changer” materials. Among these materials, the most promising category for large-scale production and application in industry are graphene oxide based materials, but some of their properties are still not well understood. Here this thesis focuses on investigating the chemical and thermochemical properties of graphene oxide based materials with both experimental and theoretical approaches. These properties are found closely related to materials chemical structures, more specifically the functional groups of the materials at the molecular level. For example, the conjugated π domain determines their capability to scavenge free radicals; the hydroxyl and carboxyl groups determine the dispersibility in aqueous or polar solvents; the epoxy groups determine the exothermic nature of the graphene oxide pyrolysis; the carbon backbone determines the reducing capability at high temperature. With the knowledge learned in this study, their implications for safe processing and storage were investigated using numeric simulations. New potential applications like oxidation protection using the antioxidant properties of the π conjugated domain and multifunctional platform for theranostics or pollutant cleanup using a couple of the unique properties of graphene oxide have been proposed and explored.
Subject
Topic
graphene oxide
Subject
Topic
processing safety
Subject (FAST) (authorityURI="http://id.worldcat.org/fast", valueURI="http://id.worldcat.org/fast/1149812")
Topic
Thermochemistry
Record Information
Record Content Source (marcorg)
RPB
Record Creation Date (encoding="iso8601")
20160629
Language
Language Term: Code (ISO639-2B)
eng
Language Term: Text
English
Identifier: DOI
10.7301/Z0B56H45
Access Condition: rights statement (href="http://rightsstatements.org/vocab/InC/1.0/")
In Copyright
Access Condition: restriction on access
Collection is open for research.
Type of Resource (primo)
dissertations