Title Information
Title
Kinetics and the Folding of RNA and Other Polymers
Name: Personal
Name Part
Zhou, Guangyao
Role
Role Term: Text
creator
Name: Personal
Name Part
Geman, Stuart
Role
Role Term: Text
Advisor
Name: Personal
Name Part
Lawrence, Charles
Role
Role Term: Text
Reader
Name: Personal
Name Part
Menon, Govind
Role
Role Term: Text
Reader
Name: Corporate
Name Part
Brown University. Department of Applied Mathematics
Role
Role Term: Text
sponsor
Origin Information
Copyright Date
2019
Physical Description
Extent
, None p.
digitalOrigin
born digital
Note: thesis
Thesis (Ph. D.)--Brown University, 2019
Genre (aat)
theses
Abstract
In this thesis, we study kinetics and the folding of RNAs and other polymers. In the first part, we study the problem from a statistical perspective. Thinking kinetically, we introduce quantitative measures of ``ambiguity" and demonstrate their statistical relationships to native secondary structure and to qualitative distinctions between RNA families. In the second part, we focus on entropic barriers in molecular dynamics simulations. Entropic barriers, while ubiquitous and important in molecular dynamics, received relatively little attention in the literature, and their theoretical characterization and understanding are severely lacking. Here, using a simple toy model with a golf-course energy landscape and two targets, we look at entropic barriers from the perspective of hitting probabilities of the targets. We present rigorous theoretical results to establish global, approximately constant hitting probabilities as an essential feature of entropic barriers, and connect the global hitting probabilities to local information around the targets (in the form of capacities of local sets around the targets) to facilitate the understanding of entropic barriers. Inspired by the theoretical results, a method called Capacity Hopping (CHop for short), based on an efficient capacity estimation algorithm, is proposed for overcoming entropic barriers in molecular dynamics simulations. Extensive numerical experiments on a concrete 5-dimensional version of the toy model show that CHop is highly effective: it can be nearly as accurate as naive simulations in terms of estimating hitting probabilities, but 750 times faster.
Subject (fast) (authorityURI="http://id.worldcat.org/fast", valueURI="http://id.worldcat.org/fast/01086244")
Topic
RNA
Subject (fast) (authorityURI="http://id.worldcat.org/fast", valueURI="http://id.worldcat.org/fast/01079687")
Topic
Protein folding
Subject (fast) (authorityURI="http://id.worldcat.org/fast", valueURI="http://id.worldcat.org/fast/01024778")
Topic
Molecular dynamics
Subject
Topic
entropic barriers
Language
Language Term (ISO639-2B)
English
Record Information
Record Content Source (marcorg)
RPB
Record Creation Date (encoding="iso8601")
20190603
Identifier: DOI
10.26300/gn9j-5d68
Access Condition: rights statement (href="http://rightsstatements.org/vocab/InC/1.0/")
In Copyright
Access Condition: restriction on access
Collection is open for research.
Type of Resource (primo)
dissertations